As strange as this is going to seem, I think the reason I think this is entirely because of Tom. He wasn't exactly sure of himself when he did Thor. But since Thor (and the movies in between) he's come into himself and I think it really shows in his acting.
I agree with bri-marie and NordicVeronica, there was definitely a noticeable in confidence levels in acting as that character. Oh and the hair... i think it just made him look a little more 'wild' or 'villain-looking'- rather than previously in Thor when his hair was predominantly slicked back with minor flicks which didn't do much for his sharp facial features like it did in the Avengers (i sound like such a fan girl here... -_-)
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